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Hydride formation in core-shell alloyed metal nanoparticles

Vladimir P. Zhdanov (Institutionen för fysik (Chalmers))
Chemical Physics Letters (0009-2614). Vol. 655-656 (2016), p. 110-114.
[Artikel, refereegranskad vetenskaplig]

The model and analysis presented are focused on hydride formation in nanoparticles with a Pd shell and a core formed by another metal. The arrangement of metal atoms is assumed to be coherent (no dislocations). The lattice strain distribution, elastic energy, and chemical potential of hydrogen atoms are scrutinized. The slope of the chemical potential (as a function of hydrogen uptake) is demonstrated to decrease with increasing the core volume, and accordingly the critical temperature for hydride formation and the corresponding hysteresis loops are predicted to decrease as well.

Nyckelord: Alloys, Hydride, Nanostructures, Strain, Stress



Denna post skapades 2016-07-05. Senast ändrad 2016-07-06.
CPL Pubid: 238999

 

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Institutionen för fysik (Chalmers)

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Fysik

Chalmers infrastruktur