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Innovative oxygen carriers uplifting chemical-looping combustion,Chemical-looping combustion, natural gas, integrated project, oxygen carrier development

Tobias Mattisson (Institutionen för energi och miljö, Energiteknik) ; J. Adánez ; K. Mayer ; F.M.M. Snijkers ; G. Williams ; E. Wesker ; O. Bertsch ; Anders Lyngfelt (Institutionen för energi och miljö, Energiteknik)
Energy Procedia: 12th International Conference on Greenhouse Gas Control Technologies, GHGT 2014; University of Texas at AustinAustin; United States; 5 October 2014 through 9 October 2014 (1876-6102). Vol. 63 (2014), p. 113-130.
[Konferensbidrag, refereegranskat]

This paper reports on the main results of the EU-financed project INNOCUOUS (Innovative Oxygen Carriers Uplifting Chemical-Looping Combustion). The project follows a series of successful projects with the aim of developing chemical-looping combustion (CLC) with gaseous fuels rich in methane. The project has included a wide range of experimental and modelling tasks, which included i) extensive screening of spray-dried and impregnated oxygen carriers, ii) production of impregnated and spray-dried oxygen carriers at >100 kg scale, iii) operation of several oxygen carriers at industrial conditions up to 120 kW scale and iv) techno-economic study of the next-scale CLC. One area of focus in the project has been the search for viable oxygen carriers which have low or no Ni. A large portfolio of interesting metal oxide systems has been found. Two oxygen carriers of CaMnxTiyMg1-x-yO3 were successfully produced in larger amounts by spray-drying and an oxygen carrier of Fe2O3/Al2O3 was produced in similar quantity using impregnation. The Ca-based material showed excellent behavior in a 10 kW and 120 kW unit, where complete combustion was achieved. With respect to the aim of replacing the bench-mark Ni-based material the project was thus very successful, as complete combustion has never been achieved in these units using Ni-based material.

Nyckelord: Chemical-looping combustion; natural gas; integrated project; oxygen carrier development

Denna post skapades 2015-03-03. Senast ändrad 2016-04-28.
CPL Pubid: 213359


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Institutionen för energi och miljö, Energiteknik (2005-2017)



Chalmers infrastruktur