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On the high-gasification rate of Brazilian manganese ore in chemical-looping combustion (CLC) for solid fuels

Peter Frohn ; Mehdi Arjmand (Institutionen för kemi- och bioteknik, Oorganisk miljökemi) ; Golnar Azimi (Institutionen för kemi- och bioteknik, Oorganisk miljökemi) ; Henrik Leion (Institutionen för kemi- och bioteknik, Oorganisk miljökemi) ; Tobias Mattisson (Institutionen för energi och miljö, Energiteknik) ; Anders Lyngfelt (Institutionen för energi och miljö, Energiteknik)
AIChE Journal (0001-1541). Vol. 59 (2013), 11, p. 4346–4354.
[Artikel, refereegranskad vetenskaplig]

The high rate of char gasification observed when using a Brazilian manganese ore as compared to ilmenite is investigated in a batch fluidized-bed reactor. Experiments were carried out at 970°C using petroleum coke, coal and wood char as fuel with a 50% H2O in N2 as fluidizing gas. A manufactured manganese oxygen carrier was also used, however, which presented a slower char conversion rate than the manganese ore. It is concluded that decrease in H2 inhibition and oxygen release are unlikely to be the main responsible mechanisms for the ore's unexpected gasification rate. The ore was also mixed in different ratios with ilmenite and it was observed that the presence of even small amounts of ore in the bed resulted in increased gasification rate. Thus, the high-gasification rate for the manganese ore could be due to a contribution from the impurities in the ore by catalyzing the gasification reaction.

Nyckelord: CO2-capture;chemical-looping combustion (CLC);manganese ore;ilmenite;solid fuels

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Denna post skapades 2013-06-30. Senast ändrad 2017-10-03.
CPL Pubid: 179540


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Institutioner (Chalmers)

Institutionen för kemi- och bioteknik, Oorganisk miljökemi (2005-2014)
Institutionen för energi och miljö, Energiteknik (2005-2017)


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